卫延召1,宋志华2,奇瑞3,王伟4,龚德瑜1,王峰5
Wei Yan-Zhao1,Song Zhi-Hua2,Qi Rui3,Wang Wei4,Gong De-Yu1,Wang Feng5
摘要: 陆梁隆起东部地区是准噶尔盆地天然气勘探的主战场。目前,在滴南凸起及周缘已经发现了一批大、中型气田(藏)。位于滴南凸起以北的滴北凸起被多个生烃凹陷环绕,发育多套烃源岩层系,天然气成藏条件十分优越。研究基于滴北凸起9个天然气样品分子和稳定碳同位素组成,并与滴南凸起天然气地球化学特征开展对比研究,结合主要烃源岩层系的埋藏史和生烃史,全面系统地梳理了滴北凸起天然气成因来源及遭受的次生改造作用。滴北凸起天然气的成因来源复杂,主要存在3类天然气:第一类是上石炭统巴山组煤系烃源岩生成的高熟煤成气;第二类是下石炭统姜巴斯套组/松喀尔苏组海相烃源岩在高成熟阶段生成的油型气;第三类是原油遭受生物降解后形成的次生生物甲烷。滴北凸起原生热成因气现今处于高成熟阶段,其非烃气体含量、稳定碳同位素组成和热成熟度等特征都与滴南凸起天然气存在显著差别,天然气的成熟度与乌伦古坳陷烃源岩匹配程度更好,推断其来自乌伦古坳陷。
中图分类号:
[1]Sun P A,Wang Y C,Leng K,et al.Geochemistry and origin of natural gas in the eastern Junggar Basin,NW China[J].Marine and Petroleum Geology,2016,75:240-251.<br /> [2]Dai Jinxing.Giant Coal-Derived Gas Fields and Their Gas Source in China[M].Beijing:Science Press,2014: 266-285.<br /> 戴金星.中国煤成大气田及气源[M].北京:科学出版社,2014:266-285.<br /> [3]Wang Xulong,Zhao Mengjun,Xiang Baoli,et al.Carboniferous source rocks in the Ludong-Wucaiwan area,Junggar Basin,NW China[J].Petroleum Exploration and Development,2010,37(5):523-530.<br /> 王绪龙,赵孟军,向宝力,等.准噶尔盆地陆东—五彩湾地区石炭系烃源岩[J].石油勘探与开发,2010,37(5):523-530.<br /> [4]Li Lin,Xia Huiping,Chen Shijia,et al.Natural gas origin and its accumulation feature in Dibei Uplift in Junggar Basin[J].Xinjiang Petroleum Geology,2010,31(4):352-355.<br /> 李林,夏惠平,陈世加,等.准噶尔盆地滴北凸起天然气成因及成藏特征[J].新疆石油地质,2010,31(4):352-355.<br /> [5]Chen Shijia,Chen Xue,Lu Jungang,et al.Characteristics of natural gas sources and accumulation in Dibei Uplift of Junggar Basin[J].Natural Gas Geoscience,2011,22(1):97-101.<br /> 陈世加,陈雪,路俊刚,等.准噶尔盆地滴北凸起天然气来源及成藏特征[J].天然气地球科学,2011,22(1):97-101.<br /> [6]Dai J X,Zou C N,Li J,et al.Carbon isotopes of Middle-Lower Jurassic coal derived alkane gases from the major basin of northwestern China[J].International Journal of Coal Geology,2009,80:124-134.<br /> [7]Wang Xulong,Zhi Dongming,Wang Yutao,et al.Organic Geochemistry of Source Rocks and Hydrocarbons in the Junggar Basin[M].Beijing:Petroleum Industry Press,2013:18-73.<br /> 王绪龙,支东明,王屿涛,等.准噶尔盆地烃源岩与油气地球化学[M].北京:石油工业出版社,2013:18-73.<br /> [8]Gong D Y,Li J Z,Ablimit I,et al.Geochemical characteristics of natural gases related to Late Paleozoic coal measures in China[J].Marine and Petroleum Geology,2018,96:474-500.<br /> [9]Graham S A,Brassel S C,Carroll A R,et al.Characteristics of selected petroleum-source rocks,Xinjiang Uygur Autonomous region,northwest China[J].AAPG Bulletin,1990,74:493-512.<br /> [10]He Dengfa,Zhang Lei,Wu Songtao,et al.Tectonic evolution stages and features of the Junggar Basin[J].Oil & Gas Geology,2018,39(5):845-861.<br /> 何登发,张磊,吴松涛,等.准噶尔盆地构造演化阶段及其特征[J].石油与天然气地质,2018,39(5):845-861.<br /> [11]Yu S,Wang X L,Xiang B L,et al.Organic geochemistry of Carboniferous source rocks and their generated oils from the eastern Junggar Basin,NW China[J].Organic Geochemistry,2014,77:72-88.<br /> [12]Gong D Y,Song Y,Wei Y Z,et al.Geochemical characteristics of Carboniferous coaly source rocks and natural gases in the southeastern Junggar Basin,NW China:Implications for new hydrocarbon explorations[J].International Journal of Coal Geology,2019,202:171-189.<br /> [13]Li Jian,Jiang Zhenglong,Luo Xia,et al.Geochemical characteristics of coal-measure source rocks and coal-derived gas in Junggar Basin,NW China[J].Petroleum Exploration and Development,2009,36(3):365-374.<br /> 李剑,姜正龙,罗霞,等.准噶尔盆地煤系烃源岩及煤成气地球化学特征[J].石油勘探与开发,2009,36(3):365-374.<br /> [14]Zhao Wenzhi,Liu Wenhui.Preliminary Study on the Accumulation and Distribution of Effective Gas Reservoirs[M].Beijing:Science Press,2008.<br /> 赵文智,刘文汇.高效天然气藏形成分布与凝析、低效气藏经济开发的基础研究[M].北京:科学出版社,2008.<br /> [15]Liu Wenhui,Xu Yongchang.A two stage model of carbon isotopic fractionation in coal gas[J].Geochimica,1999,28(4):359-366.<br /> 刘文汇,徐永昌.煤成气碳同位素演化二阶段分馏模式及机理[J].地球化学,1999,28(4):359-366.<br /> [16]Bernard B B,Brooks J M,Sackett W M.Light hydrocarbons in recent Texas continental shelf and slope sediments[J].Journal of Geophysical Research,1978,83:4053-4061.<br /> [17]Whiticar M J.Correlation of natural gases with their sources[C]∥Magoon L,Dow W.The Petroleum System-From Source to Trap[J].New York:AAPG Memoir,1994,60:261-284.<br /> [18]Dai Jinxing,Pei Xigu,Qi Houfa.China Natural Gas Geology(Vol.1)[M].Beijing:Petroleum Industry Press,1992:65-87.<br /> 戴金星,裴锡古,戚厚发.中国天然气地质学(卷一)[M].北京:石油工业出版社,1992:65-87.<br /> [19]Jenden P D,Kaplan I R,Poreda R.Origin of nitrogen-rich natural gases in the California Great Valley:Evidence from helium,carbon and nitrogen isotope ratios[J].Geochimica et Cosmochimica Acta,1988,52:851-861.<br /> [20]Rooney M,Claypool G,Chung H.Modeling thermogenic gas generation using carbon isotope ratios of natural gas hydrocarbons[J].Chemical Geology,1995,126:219-232.<br /> [21]Berner U,Faber E.Empirical carbon isotope/maturity relationships for gases from algal kerogens and terrigenous organic matter,based on dry,open-system pyrolysis[J].Organic Geochemistry,1996,24:947-955.<br /> [22]Berner U,Faber E,Scheeder G,et al.Primary cracking of a1gal and landplant kerogens:Kinetic models of isotope variations in methane,ethane and propane[J].Chemical Geology,1995,126(3):233-245.<br /> [23]Milkov A V.Worldwide distribution and significance of secondary microbial methane formed during petroleum biodegradation in conventional reservoirs[J].Organic Geochemistry,2011,42:184-207.<br /> [24]Dai J X,Gong D Y,Ni Y Y,et al.Stable carbon isotopes of coal-derived gases sourced from the Mesozoic coal measures in China[J].Organic Geochemistry,2014,74:123-142.<br /> [25]Dai J X,Ni Y Y,Zou C N.Stable carbon and hydrogen isotopes of natural gases source from the Xujiahe Formation in the Sichuan Basin,China[J].Organic Geochemistry,2012,43(1):103-111.<br /> [26]Liang D G,Zhang S C,Chen J P,et al.Organic geochemistry of oil and gas in the Kuqa Depression,Tarim Basin,NW China[J].Organic Geochemistry,2003,34:873-888.<br /> [27]Gang Wenzhe,Gao Gang,Hao Shisheng,et al.Carbon isotope of ethane applied in the analyses of genetic types of natural gas[J].Petroleum Geology & Experiment,1997,19(2):164-167.<br /> 刚文哲,高岗,郝石生,等.论乙烷碳同位素在天然气成因类型研究中的应用[J].石油实验地质,1997,19(2):164-167.<br /> [28]Tissot B P,Pelet R,Ungerer P H.Thermal history of sedimentary basins,maturation indices and kinetics of oil and gas generation[J].AAPG Bulletin,1987,71:1445-1466.<br /> [29]Law B E,Rice D D.Hydrocarbons from Coal[C].American Association of Petroleum Geologists Studies in Geology,1993,38:133-158.<br /> [30]Petersen H I.A re-consideration of the“oil window” for humic coal and kerogen type Ⅲ source rocks[J].Journal of Petroleum Geology,2006,24:407-432.<br /> [31]Petersen H I,Nytoft H P.Oil generation capacity of coals as a function of coal age and aliphatic structure[J].Organic Geochemistry,2006,37:558-583.<br /> [32]He Sheng.Wulungu region in Junggar Basin Carboniferous source characteristics and potential of oil and gas[J].Science Technology and Engineering,2017,17(2):162-166.<br /> 何胜.准噶尔盆地乌伦古地区石炭系油气源特征及潜力探讨[J].科学技术与工程,2017,17(2):162-166.<br /> [33]Zhang Lin,Du Xiaodi,Li Feng,et al.Hydrocarbon source rocks evaluation of the Wulungu Depression,Junggar Basin[J].China Mining Magazine,2016,25(9):141-147.<br /> 张林,杜小弟,李锋,等.准噶尔盆地乌伦古坳陷主力烃源岩分析[J].中国矿业,2016,25(9):141-147.<br /> [34]George S C,Boreham C J,Minifie S A,et al.The effect of minor to moderate biodegradation on C<sub>5</sub> to C<sub>9 </sub>hydrocarbons in crude oils[J].Organic Geochemistry,2002,33:1293-1317.<br /> [35]Gong D Y,Ma R L,Chen G,et al.Geochemical characteristics of biodegraded natural gas and its associated low molecular weight hydrocarbons[J].Journal of Natural Gas Science and Engineering,2017,46:338-349.<br /> [36]Welte D H,Kratochvil H,Rullktter H,et al.Organic geochemistry of crude oils from the Vienna Basin and an assessment of their origin[J].Chemical Geology,1982,35:33-68.<br /> [37]Tao K Y,Jian Cao J,Wang Y C,et al.Geochemistry and origin of natural gas in the petroliferous Mahu Sag,northwestern Junggar Basin,NW China:Carboniferous marine and Permian lacustrine gas systems[J].Organic Geochemistry,2016,100:62-79.<br /> [38]Chen Jianping,Wang Xulong,Deng Chunping,et al.Oil and gas source,occurrence and petroleum system in the Junggar Basin,northwest China[J].Acta Geologica Sinica,2016,90(3):421-450.<br /> 陈建平,王绪龙,邓春萍,等.准噶尔盆地油气源、油气分布与油气系统[J].地质学报,2016,90(3):421-450.<br /> [39]Cao J,Wang X L,Sun P A,et al.Geochemistry and origins of natural gases in the central Junggar Basin,northwest China[J].Organic Geochemistry,2012,53:166-176.<br /> [40]Chen Z H,Cao Y C,Ma Z J,et al.Geochemistry and origins of natural gases in the Zhongguai area of Junggar Basin,China[J].Journal of Petroleum Science and Engineering,2014,119:17-27.<br /> <div> <br /> </div> |
[1] | 戴金星, 洪峰, 倪云燕, 廖凤蓉. 塔里木盆地英吉苏凹陷煤成气前景良好[J]. 天然气地球科学, 2019, 30(6): 771-782. |
[2] | 秦胜飞, 白斌, 袁苗, 周国晓, 杨晋东. 四川盆地中部地区海相储层煤成气来源[J]. 天然气地球科学, 2019, 30(6): 790-797. |
[3] | 胡自龙, 卞保力, 刘海磊, 赵龙, 卢山, 王绍清. 准噶尔盆地大井地区天然气成因、来源与成藏过程[J]. 天然气地球科学, 2019, 30(6): 850-859. |
[4] | 李剑, 郝爱胜, 齐雪宁, 陈旋, 国建英, 冉启贵, 李志生, 谢增业, 曾旭, 李谨, 王瑀, 刘如红, . 中国西北地区侏罗系煤成气地球化学特征与勘探潜力[J]. 天然气地球科学, 2019, 30(6): 866-879. |
[5] | 胡瀚文, 张元元, 卓勤功, 贾承造, 郭召杰. 准噶尔盆地南缘下组合油气成藏过程——以齐古油田为例[J]. 天然气地球科学, 2019, 30(4): 456-467. |
[6] | 付爽, 庞雷, 许学龙, 曹元婷, 刘振宇, 张顺存, . 准噶尔盆地玛湖凹陷下乌尔禾组储层特征及其控制因素[J]. 天然气地球科学, 2019, 30(4): 468-477. |
[7] | 王伟锋, 张仲达. 准噶尔盆地五彩湾地区石炭系烃源岩演化及油气成藏过程[J]. 天然气地球科学, 2019, 30(4): 447-455. |
[8] | 潘建国, 黄林军, 王国栋, 郭娟娟, 马永平, 罗昭洋. 源外远源油气藏的内涵和特征——以准噶尔盆地盆1井西富烃凹陷为例[J]. 天然气地球科学, 2019, 30(3): 312-321. |
[9] | 高崇龙,纪友亮,靳军,王剑,任影,曾力,王道伟,张昊,李谨杰. 古隆起埋藏期沟谷残丘地貌下沉积体系及油气藏发育模式——以准噶尔盆地腹部石南地区清水河组一段为例[J]. 天然气地球科学, 2018, 29(8): 1120-1137. |
[10] | 裴立新,刚文哲,朱传真,刘亚洲,何文军,向宝力,董岩. 准噶尔盆地烷烃气碳同位素组成及来源[J]. 天然气地球科学, 2018, 29(7): 1020-1030. |
[11] | 王国龙,杜社宽. 准噶尔盆地北三台凸起二叠系梧桐沟组一段碎屑岩储层特征及控制因素[J]. 天然气地球科学, 2018, 29(5): 675-681. |
[12] | 何文军,杨海波,费李莹,王学勇,杨彤远,杨翼波,鲍海娟. 准噶尔盆地新光地区佳木河组致密砂岩气有利区资源潜力综合分析[J]. 天然气地球科学, 2018, 29(3): 370-381. |
[13] | 王小垚,曾联波,周三栋,史今雄,田鹤. 低阶煤储层微观孔隙结构的分形模型评价[J]. 天然气地球科学, 2018, 29(2): 277-288. |
[14] | 石新朴, 覃建强, 丁艳雪, 杨丹, 史全党, 胡清雄, 李波, 齐洪岩, 张吉辉, 孙德强, 赵振, 饶远, 习成威. 准噶尔盆地滴南凸起火山岩气藏成藏主控因素与成藏模式[J]. 天然气地球科学, 2018, 29(12): 1706-1714. |
[15] | 杨海波, 王屿涛, 郭建辰, 何文军, 蓝文芳. 准噶尔盆地天然气地质条件、资源潜力及勘探方向[J]. 天然气地球科学, 2018, 29(10): 1518-1530. |
|