CHEN Rui-yin，WANG Hui-tong，CHEN Jian-ping，LIU Yu-ying . An Experimental Method to Evaluate the Hydrocarbon Generationand Expulsion Efficiency in the Songliao Basin[J]. Natural Gas Geoscience, 2015 , 26(5) : 915 -921 . DOI: 10.11764/j.issn.1672-1926.2015.05.0915

［1］Pang Xiongqi.Modeling of Geologic Process［M］.Beijing:Petroleum Industry Press,2003:1-487.［庞雄奇.地质过程定量模拟［M］.北京:石油工业出版社,2003:1-487.］
［2］Hu Qingming.Exploration and development of shale gas in China achieving a major breakthrough[J].Energy Conservation in Petroleum & Petrochemical Industry,2014,4(11):52.［胡庆明.我国页岩气勘探开发实现重大突破[J].石油石化节能,2014,4(11):52.］
［3］Wu Xin,Ren Zhiyong,Wang Yong,et al.Situation of world shale gas exploration and development[J].Resources & Industry,2013,15(5):61-67.［吴馨,任志勇,王勇,等.世界页岩气勘探开发现状[J].资源与产业,2013,15(5):61-67.］
［4］Yu Guoming,Xu Xu.Shale gas in Fuling:Historical breakthrough[J].China Petrochemical Industry,2014,(4):13-16.［俞国明,徐徐.涪陵页岩气:历史性突破[J].中国石化,2014,(4):13-16.］
［5］Guo Wei,Yu Wenxiang,Liu Zhaojun,et al.The burial history of the southern Songliao Basin[J].Journal of Jilin University:Earth Science Edition,2009,39(3):353-360.［郭崴,宇文祥,刘招君,等.松辽盆地南部埋藏史[J].吉林大学学报:地球科学版,2009,39(3):353-360.］
［6］Lewan M D.Laboratory Simulation of Petroleum Formation Hydrous Pyrolysis［M］.Organic geochemistry,edited by Michael H.Engel and Stephen A.Macko.New York:Plenum Press,1993:419-440.
［7］Zheng Lunju,Qin Jianzhong,He Sheng,et al.Preliminary study of formation porosity thermo compression simulation experiment of hydrocarbon generation and expulsion[J].Petroleum Geology & Experiment,2009,31(3):296-302.［郑伦举,秦建中,何生,等.地层孔隙热压生排烃模拟实验初步研究[J].石油实验地质,2009,31(3):296-302.］
［8］Qian Zhihao,Cao Yulan,Rong Zhengguang.Light hydrocarbon determination with thermal evaporation method[J].Petroleum Geology & Experiment,1982,4(4):280-284.[JP3]［钱志浩,曹玉兰,荣正光.热蒸发法测定轻烃[J].石油实验地质,1982,4(4):280-284.］
［9］Qian Zhihao,Cao Yin,Wang Congfeng,et al.The New Progress of Petroleum Geological Test Technology［M］.Beijing:Geological Publishing House,1994:1-194.[JP3]［钱志浩,曹寅,王从风,等.石油地质实验测试技术新进展［M］.北京:地质出版社,1994:1-194.］
[10]Qin Jianzhong,Qian Zhihao,Cao Yin,et al.New techniques in oil and gas geochemical exploration[J].Petroleum Geology & Experiment,2005,27(5):519-528.［秦建中,钱志浩,曹寅,等.油气地球化学新技术新方法[J].石油实验地质,2005,27(5):519-528.］
［11］Liu Weixin,Ba Liqiang,Zhang Meizhen,et al.New technological advances in petroleum exploration[J].Petroleum Geology & Experiment,2003,25(6):777-782.［刘伟新,把立强,张美珍,等.石油地质分析测试技术新进展[J].石油实验地质,2003,25(6):777-782.］
［12］Jiang Qigui,Chen Weijun,Jin Juchang,et al.Analysis method of light hydrocarbon with low boiling-point from source rocks[J].Petroleum Geology & Experiment,2004,26(5):492-495.［蒋启贵,陈伟钧,金聚畅,等.岩石低沸点轻烃指纹分析方法研究[J].石油实验地质,2004,26(5):492-495.］
［13］Jiang Qigui,Zhang Caiming,Zhang Meizhen,et al.Research on the quantitative analysis method of C₆-C₁₅ light hydrocarbon in source rock samples[J].Petroleum Geology & Experiment,2007,29(5):512-521.［蒋启贵,张彩明,张美珍,等.岩石C₆-C₁₅轻烃定量分析方法研究[J].石油实验地质,2007,29(5):512-521.］
［14］Xiong Yongqiang,Geng Ansong,Wang Yunpeng,et al.Experimental research of kerogen secondary hydrocarbon generation kinetics[J].Science in China:Series D,2001,31(4):315-320.［熊永强,耿安松,王云鹏,等.干酪根二次生烃动力学模拟实验研究[J].中国科学:D辑,2001,31(4):315-320.］
［15］Wang Huitong,Zhang Shuichang,Weng Na,et al.Analysis of condensate oil by comprehensive two-dimensional gas chromatography[J].Petroleum Exploration and Development,2012,39(1):123-128.［王汇彤,张水昌,翁娜,等.凝析油全二维气相色谱分析[J].石油勘探与开发,2012,39(1):123-128.］
［16］Adahchour M,Beens J,Vreuls R J J,et al.Recent developments in comprehensive two-dimensional gas chromatography(GC×GC):Introduction and instrumental setup[J].Trends in Analytical Chemistry,2006,25(5):438-454.
［17］Reddy C M,Nelson R K,Sylva S,et al.Identification and quantification of alkene-based drilling fluids in crude oils by comprehensive two-dimensional gas chromatography with flame ionization detection[J].Journal of Chromatography A,2007,1148(1):100-107.
［18］Wang Zhaoyun,Cheng  Keming,Zhang Baisheng,et al.The study on simulation experiments of hydrocarbon generation and expulsion of mud limestone[J].Acta Sedimentologica Sinica,1996,14(1):127-134.［王兆云,程克明,张柏生,等.泥灰岩的生排烃模拟实验研究[J].沉积学报,1996,14(1):127-134.］
［19］Hao Fang.Kinetics of Hydrocarbon Generation and Mechanisms of Petroleum Accumulation in Overpressured Basins［M］.Beijing:Science Press,2005:1-406.［郝芳.超压盆地生烃作用动力学与油气成藏机理［M］.北京:科学出版社,2005:1-406.］
［20］Chen Jianyu,Hao Fang.Improvement of organic petrology studying types and maturity of organic matter[J］.Petroleum Geology and Experiment,1990,12(4):426-431.［陈建渝,郝芳.有机岩石学研究有机质类型和成熟度的改进[J].石油实验地质,1990,12(4):426-431.］
[21]Jones R W,Edison T A.Microscopic observations of kerogen related to geochemical parameters with emphasis on thermal [JP3]maturation［M］//Oltz D F.Low Temperature Metamorphism of Kerogen and Clay Minerals:SEPM,Los Angeles:Pacific Section,1978:1-12.
［22］Horsfield B.Practical criteria for classifying kerogens:Some observations from pyrolysis-gas chromatography[J].Geochim Cosmochim Acta,1989,53(4):891-901.
［23］Baskin D K.Atomic H/C ratio of kerogen as an estimate of thermal maturity and organic matter conversion[J］.AAPG Bulletin,1997,8l (9):1437-1450.
［24］Braun R L,Burnham A K.Mathematical model of oil generation,degradation and expulsion[J].Energy Fuels,1990,4(1):132-146.
［25］Chandra D.Reflectance of coals carbonized under pressure[J].Economic Geology,1965,60(3):621-629.
［26］Hryckowian E,Dutcher R R,Dachille F.Experimental studies of anthracite coals at high pressures and temperatures[J].Economic Geology,1967,62(4):517-539.
［27］Yang Tianyu,Wang Hanyun.Simulation experiment of organic matter in high temperature and high pressure[J］.Petroleum Geology & Experiment,1987,8(4):380-389.［杨天宇,王涵云.岩石中有机质高温高压模拟实验[J].石油与天然气地质,1987,8(4):380-389.］
［28］Huang Jianquan,Zhou Zhongyi,Fan  Shanfa.High Temperature and High Pressure Experimental Study on the Formation of Deep Basin Petroleum[M］.Nanjing:Jiangsu Science & Technology Press,1992:244-245.［黄健全,周中毅,范善发.盆地深部油气形成的高温高压实验研究［M］.南京:江苏科学技术出版社,1992:244-245.］
［29］Xie Qilai,Fan Shanfa,Zhou Zhongyi.Simulation experiment of pressure affecting on evolution and hydrocarbon generation of source rock[J].Mineral Rock Geochemistry Bulletin,1996,15(2):91-93.［解启来,范善发,周中毅.压力对烃源层演化及产烃影响的模拟实验[J].矿物岩石地球化学通报,1996,15(2):91-93.］
［30］Sajgo C S,Mcevoy J,Wolef G A,et al.Influence of temperature and pressure on maturation process[J].Organic Geochemistry,1986,10(1-3):331-337.
［31］Price L C,Wenger L M.The influence of pressure on petroleum generation and maturation as suggested by aqueous pyrolysis[J].Organic Geochemistry,1992,19(1-3):141-159.
［32］Dalla Torre M,Mahlmann R F,Ernst W G.Experimental study on the pressure dependence of vitrinite maturity[J].Organic Geochemistry,1997,61(4):2921-2928.
［33］Jiang Feng,Du Jianguo,Wang Wanchun,et al.Research on ultra high pressure high temperature simulation experiments:The influence of high temperature and pressure on organic matter maturation[J].Acta Sedimentologica  Sinica,1998,16(3):153-160.［姜峰,杜建国,王万春,等.高温超高压模拟实验研究:温压条件下对有机质成熟作用的影响[J].沉积学报,1998,16(3):153-160.］
［34］Hao Fang,Jiang Jianqun,Zou huayao,et al.The overpressure differently and levelly retard the organic matter evolution[J].Science in China:Series D,2004,34(5):443-451.
［35］Sweeney J J,Burnham A K,Braun R L.A model of hydrocarbon generation from type one kerogen:Application to Uninta basin,Utah[J].AAPG Bulletin,1987,71(8):967-985.
［36］Xiao Zhihua,Hu Guoyi,Li Zhisheng.Effect of pressure on hydrocarbon generation of source rock in close system[J].Natural Gas Geoscience,2007,18(2):284-288.［肖芝华,胡国艺,李志生.封闭体系下压力变化对烃源岩产气率的影响[J].天然气地球科学,2007,18(2):284-288.］
［37］Zhou Lihong,Yu Xuemin,Jiang Wenya,et al.Overpressure retardation of the thermal evolution of Paleogene source rocks and its significance for petroleum geology in Qikou Sag[J].Natural Gas Geoscience,2013,24(6):1118-1124.［周立宏,于学敏,姜文亚,等.歧口凹陷异常压力对古近系烃源岩热演化的抑制作用及其意义[J].天然气地球科学,2013,24(6):1118-1124.］